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  1. The scientific case for concurrent neutron and X-ray scattering and spectroscopy

    The interrogation of materials with X-rays or neutrons to determine structure, energetics, and dynamics is fundamental to advancing physical and chemical materials science and enabling innovative material technologies. A persistent challenge in materials development is that progress depends on understanding structure and dynamics across multiple length and time scales in increasingly complex, multicomponent systems featuring interfaces, heterogeneity, and hierarchical organization. Despite rapidly growing demands on materials characterization, current experimental approaches are almost exclusively based on isolated X-ray or neutron scattering and spectroscopy, reflecting a paradigm largely unchanged for decades. To assess the scientific need for a new experimental paradigm, amore » 3-day workshop sponsored by the U.S. National Science Foundation (NSF) was held at the SpringHill Suites, San Jose, California, from June 2 to 4, 2022. The workshop brought together 70 national and international experts who critically evaluated opportunities enabled by concurrent neutron and X-ray (NeX) scattering, spectroscopy, and imaging experiments. The participants reached a clear consensus that establishing NeX capabilities is crucial for advancing the science of complex materials in the United States. This report illustrates the scientific drivers for NeX experiments through representative examples spanning biomaterials, energy materials, soft matter, nanomaterials, quantum materials, geoscience, and applied materials research. The complementarity of neutrons and X-rays is essential for robust model development and refinement, particularly in multiphase and multicomponent systems. While joint refinement of data from separate experiments is valuable, concurrent measurements uniquely eliminate uncertainties arising from sample evolution, environmental drift, and irreproducibility associated with experiments performed at different locations and times. Realizing NeX capabilities will require the development of new instrumentation, data analysis frameworks, and robust sample environments compatible with both neutron and X-ray probes. Addressing these challenges will enable unambiguous interpretation of complex materials behavior and open new frontiers in materials research.« less
  2. A Brief Review of the Impact of Neutron Irradiation Damage in Tungsten and Its Alloys

    Neutron irradiation poses a substantial challenge in the development and application of tungsten (W) and its alloys, predominantly in the framework of nuclear fusion and fission environments. Although W is well-acknowledged for its unique properties like its high melting temperature and higher resistance to sputtering, transmutation products, such as Re and Os, form and impact the alloy properties as a result of neutron irradiation. This transmutation effect accompanied by significant microstructure damage due to neutron irradiation can lead to the significant degradation of mechanical properties. This review surveys the literature focusing on the microstructural modifications post-irradiation and its impacts onmore » the irradiation hardening. This review provides insights into the elaborative understanding on the neutron radiation damage on W and W alloys by exploring the microstructural evolution and hardness changes post-irradiation. The gaps and future opportunities for understanding neutron radiation damage in W are briefly summarized.« less
  3. Quantification of the light output anistropy in deuterated stilbene

    Deuterated stilbene is an organic scintillator that is a desirable material for fast neutron spectroscopy using spectrum unfolding techniques without requiring time-of-flight information. Due to the crystal structure of the material, some anisotropy of the light output exists, which is dependent on the direction of heavy charged particle recoil relative to the crystal structure. The anisotropy of trans-stilbene (hereafter referred to as stilbene) has been well characterized in previous work, but for deuterated stilbene, the anisotropy has only been partially characterized along the a and b crystal axes, while the artificial c' axis, which shows the largest anisotropy in stilbene,more » has not been characterized until this publication. Here, in this work, two deuterated stilbene crystals were characterized with neutron energies up to 35 MeV at the Los Alamos Neutron Science Center. For one of the crystals, the response is characterized along the a, b, and c' axes. This characterization shows a distinct anisotropy along the axes in deuterated stilbene, which is very similar to that found in regular stilbene, such that the a axis is the brightest, while the b' and c' axes are approximately 3% and 20%–35% lower relative to the a axis.« less
  4. Observing the onset of the accretion wake in Vela X-1

    High-mass X-ray binaries (HMXBs) offer a unique opportunity to investigate accretion onto compact objects and the wind structure in massive stars. A key source for such studies is the bright neutron star HMXB Vela X-1 whose convenient physical and orbital parameters facilitate analyses and in particular enable studies of the wind structure in HMXBs. Here, we analyse simultaneous XMM-Newton and NuSTAR observations at $$\phi_{orb}$$ ≈ 0.36–0.52 and perform time-resolved spectral analysis down to the pulse period of the neutron star based on our previous NuSTAR-only results. For the first time, we are able to trace the onset of the wakesmore » in a broad 0.5–78 keV range with a high-time resolution of ~283 s and compare our results with theoretical predictions. Here we observed a clear rise in the absorption column density of the stellar wind NH,1 starting at orbital phase ~0.44, corresponding to the wake structure entering our line of sight towards the neutron star, together with local extrema throughout the observation, which are possibly associated with clumps or other structures in the wind. Periods of high absorption reveal the presence of multiple fluorescent emission lines of highly ionised species, mainly in the soft-X-ray band between 0.5 and 4 keV, indicating photoionisation of the wind.« less
  5. Advancements of the nSpec system

    For this study, a new characterization of the detector response for the EJ301 liquid scintillator based nSpec system has been conducted at the Los Alamos Neutron Science Center. The new characterization was accomplished in two orders of magnitude less time and with better statistics than the previous characterization. The new and old characterization methods were compared by conducting both types of characterization on two detectors (one EJ301 and one EJ301D). The two methods show consistent results and compare well to results previously published in the literature; however, the results from the characterization of the original nSpec detector show discrepancies thatmore » have been identified as being caused by oxygen being absorbed into the detector due to a leak. The new characterized detector response shows improved spectrum unfolding performance than the previous characterization. The cross talk of the detector system was also characterized as a function of incident neutron energy and found to have a negligible impact on spectrum unfolding results. Alternative materials (EJ301D and stilbene) were also characterized in a first step towards an upgraded system. The different materials show little difference in unfolding performance, but the comparison is ongoing. A SiPM based stilbene detector was used to evaluate the use of SiPMs in a future system upgrade. The SiPM provides adequate performance, but the custom SiPM readout results in a much longer pulse width than PMT based systems. The measured light output of the SiPM based stilbene compares well with the results in literature. Future work will look at additional materials (deuterated stilbene and organic glass) and optimizing the SiPM readout to decrease the pulse width.« less
  6. A realistic guide misalignment model for the Second Target Station instruments at the Spallation Neutron Source

    The Second Target Station (STS) at the Spallation Neutron Source, including a suite of initial instrument concepts, are being designed in Oak Ridge. The moderator size at STS is significantly smaller than that of the First Target Station, making the guide misalignment a more prominent concern. Here a realistic misalignment model based on Monte Carlo neutron ray tracing simulation was developed to evaluate the impacts of both the random misalignment and floor settlement on the performance of a toy model of 150 m straight guide system, and MENUS, an STS instrument concept with a typical guide design of two opposing Montelmore » mirrors. The study shows that longer instruments, and instruments with complex curved mirrors/guides are sensitive to significant performance penalties due to misalignments.« less
  7. Hydrodynamic simulations of electron-capture supernovae: progenitor and dimension dependence

    ABSTRACT We present neutrino-transport hydrodynamic simulations of electron-capture supernovae (ECSNe) in flash with new two-dimensional (2D) collapsing progenitor models. These progenitor models feature the 2D modelling of oxygen-flame propagation until the onset of core collapse. We perform axisymmetric simulations with six progenitor models that, at the time of collapse, span a range of propagating flame front radii. For comparison, we also perform a simulation with the same set-up using the canonical, spherically symmetrical progenitor model n8.8. We found that the variations in the progenitor models inherited from simulations of stellar evolution and flame propagation do not significantly alter the globalmore » properties of the neutrino-driven ECSN explosion, such as the explosion energy (∼1.36–1.48 × 1050 erg) and the mass (∼0.017–0.018 M⊙) and composition of the ejecta. Due to aspherical perturbations induced by the 2D flame, the ejecta contains a small amount (≲1.8 × 10−3 M⊙) of low-Ye (0.35 < Ye < 0.4) component. The baryonic mass of the protoneutron star is ∼1.34 M⊙ (∼1.357 M⊙) with the new (n8.8) progenitor models when simulations end at ∼400 ms and the discrepancy is due to updated weak-interaction rates in the progenitor evolutionary simulations. Our results reflect the nature of ECSN progenitors containing a strongly degenerate oxygen–neon–magnesium (ONeMg) core and suggest a standardized ECSN explosion initialized by ONeMg core collapse. Moreover, we carry out a rudimentary three-dimensional simulation and find that the explosion properties are fairly compatible with the 2D counterpart. Our paper facilitates a more thorough understanding of ECSN explosions following the ONeMg core collapse, though more three-dimensional simulations are still needed.« less
  8. Long-term general relativistic magnetohydrodynamics simulations of magnetic field in isolated neutron stars

    ABSTRACT Strong magnetic fields play an important role in powering the emission of neutron stars. Nevertheless, a full understanding of the interior configuration of the field remains elusive. In this work, we present general relativistic magnetohydrodynamics (MHD) simulations of the magnetic field evolution in neutron stars lasting $${\sim } {880}\,$$ms (∼6.5 Alfvén crossing periods) and up to resolutions of $$0.1155\,$$km using Athena++. We explore two different initial conditions, one with purely poloidal magnetic field and the other with a dominant toroidal component, and study the poloidal and toroidal field energies, the growth times of the various instability-driven oscillation modes, and turbulence.more » We find that the purely poloidal setup generates a toroidal field, which later decays exponentially reaching $$1{{\ \rm per\ cent}}$$ of the total magnetic energy, showing no evidence of reaching equilibrium. The initially stronger toroidal field setup, on the other hand, loses up to 20 per cent of toroidal energy and maintains this state till the end of our simulation. We also explore the hypothesis, drawn from previous MHD simulations, that turbulence plays an important role in the quasi-equilibrium state. An analysis of the spectra in our higher resolution setups reveals, however, that in most cases we are not observing turbulence at small scales, but rather a noisy velocity field inside the star. We also observe that the majority of the magnetic energy gets dissipated as heat increasing the internal energy of the star, while a small fraction gets radiated away as electromagnetic radiation.« less
  9. Theoretical Constraints on Neutron-Mirror-Neutron Oscillation

    Mirror models lead to the possibility that neutron (n) can oscillate into its mirror partner (n′), inspiring several experimental searches for this phenomenon. The condition for observability of this oscillation is a high degree of degeneracy between the n and n′ masses, which can be guaranteed if there is exact parity symmetry taking all particles to their mirror partners. However, consistency of these models with big-bang nucleosynthesis requires that this parity symmetry be broken in the early universe in a scenario called asymmetric inflation. In this paper, we study the consistency of an observable n−n′ oscillations signal with asymmetric inflationmore » and derive various theoretical constraints. In particular, we find that the reheat temperature after inflation should lie below 2.5 TeV, and we predict a singlet fermion with a mass below 100 GeV. In simple models, where the right-handed neutrino is a mediator of baryon-number-violating interactions, we find that the light neutrinos are Dirac fermions with their masses arising radiatively through one-loop diagrams.« less
  10. Fast Neutron Scintillator Screens for Neutron Imaging Using a Layered Polymer-Phosphor Architecture

    Fast neutrons enable a nondestructive examination of dense, large, and highly attenuating samples due to their lower interaction probability compared to thermal neutrons. However, this also creates a challenge in fast neutron imaging, as the thicker sensors necessary to detect fast neutrons degrade an image’s spatial resolution due to scattering within the sensor and the indeterminate depth of interaction in the sensor. This work explores the advantages of a fast neutron imaging screen with a layered polymer-phosphor screen approach as opposed to a mixed polymer-phosphor screen typically used in fast neutron imaging. Proton recoil is the primary conversion mechanism formore » fast neutron imaging. Simulations showed that the recoil proton range of typical fast neutrons is approximately 200 µm, however, tests at Idaho National Laboratory revealed that the light output of these screens increased at much greater polymer thicknesses. The NECTAR fast neutron beamline at FRM II was used to test the imaging performance of layered fast neutron imaging screens. Distinguishing between the fast-neutron and γ-ray signals is a major challenge in fast neutron imaging because all fast neutron sources also produce γ-rays. A relative comparison between a control plate and the fast neutron screen was made to distinguish between a γ-ray and fast neutron signals. MCNP modeling quantified the γ-ray and fast neutron contributions to the images measured at NECTAR, which were approximately a 75% γ-ray image.« less
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